Design of shell-type ligands for luminescent lanthanide complexes

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http://eprints.org/relation/isVolatileVersionOf http://etheses.bham.ac.uk/id/document/3910 http://eprints.org/relation/ispreviewThumbnailVersionOf http://etheses.bham.ac.uk/id/document/3910 http://eprints.org/relation/isVersionOf http://etheses.bham.ac.uk/id/document/3910 archive 4031 disk0/00/00/17/42 2011-07-07 13:16:13 2019-01-23 09:54:46 2011-07-19 16:40:58 thesis show 0 Davies Dita University of Birmingham Design of shell-type ligands for luminescent lanthanide complexes unpub QD 10col_ephy A series of lanthanide complexes based on tetraphenyl imidodiphosphate ligand have been prepared in order to investigate the ligand ability to act as a sensitiser for f-f based luminescence for the visible and NIR emitting ions. Furthermore, novel bimetallic luminescent lanthanide complexes based on two imidodiphosphate binding sites have been prepared for the examination of dinuclear lanthanide complexes formation. The sensitising properties of the bistpOp have been investigated by luminescence spectroscopy. A new ligand based on biphenyl sensitisers has been developed utilising an imidodiphosphate binding site. The lanthanide complexes have been prepared and their photophysical properties analysed. 2011-07 2010-10 graduation eng This unpublished thesis/dissertation is copyright of the author and/or third parties. The intellectual property rights of the author or third parties in respect of this work are as defined by The Copyright Designs and Patents Act 1988 or as modified by any successor legislation. Any use made of information contained in this thesis/dissertation must be in accordance with that legislation and must be properly acknowledged. Further distribution or reproduction in any format is prohibited without the permission of the copyright holder. Ubira@lists.bham.ac.uk public University of Birmingham School of Chemistry d_ph na 2011-07 graduation